Usually means: Make smooth by removing creases.
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We found 12 dictionaries that define the word unwrinkle:

General (12 matching dictionaries)
  1. unwrinkle: Merriam-Webster
  2. unwrinkle: Collins English Dictionary
  3. unwrinkle: Wordnik
  4. unwrinkle: Wiktionary
  5. unwrinkle: Infoplease Dictionary
  6. Unwrinkle, unwrinkle: Dictionary.com
  7. Unwrinkle: Online Plain Text English Dictionary
  8. unwrinkle: Webster's Revised Unabridged, 1913 Edition
  9. Unwrinkle: AllWords.com Multi-Lingual Dictionary
  10. unwrinkle: Webster's 1828 Dictionary
  11. unwrinkle: FreeDictionary.org
  12. Unwrinkle: TheFreeDictionary.com

Definitions from Wiktionary (unwrinkle)

verb:  (transitive) To remove wrinkles from.
verb:  (intransitive) To stop being wrinkly; to become flat or smooth.

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