Sorry, no online dictionaries contain the exact phrase opposite of entangle.
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Reverse dictionary results:
1. untangle
2. unravel
3. unwind
4. disentangle
5. loosen
6. deblock
7. disbranch
8. disembroil
9. disencumber
10. disentail
11. leese
12. let down
13. unanchor
14. unbrace
15. unbraid
16. unbridle
17. unbuckle
18. unbuckling
19. unbutton
20. uncenter
21. unclench
22. uncoating
23. uncouple
24. uncoupler
25. uncumber
26. uncurse
27. unencumber
28. unentangle
29. unharness
30. unhinge
31. unindent
32. unmake
33. unmask
34. unmesh
35. unmoor
36. unpark
37. unpeel
38. unpick
39. unplug

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   entangle ?
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