Usually means: Converse to attract or flirt.
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We found 19 dictionaries that define the word chat up:

General (14 matching dictionaries)
  1. chat up: Merriam-Webster
  2. chat-up: Oxford Learner's Dictionaries
  3. chat up: Collins English Dictionary
  4. chat up: Vocabulary.com
  5. chat-up: Wordnik
  6. chat up: Wiktionary
  7. chat up: Dictionary.com
  8. chat up: Rhymezone
  9. chat up: FreeDictionary.org
  10. chat up: Mnemonic Dictionary
  11. chat up: TheFreeDictionary.com
  12. chat up: Longman Dictionary of Contemporary English

Business (1 matching dictionary)
  1. chat up: Legal dictionary

Computing (1 matching dictionary)
  1. chat up: Encyclopedia

Slang (3 matching dictionaries)
  1. chat up: Green’s Dictionary of Slang
  2. chat up: English slang and colloquialisms used in the United Kingdom
  3. chat up: Urban Dictionary

Definitions from Wiktionary (chat up)

verb:  (transitive, idiomatic) To talk to (someone) in a friendly, open, or casual manner, sometimes also in a charming or affected manner, usually to curry favor, and sometimes flirtatiously with the intention of establishing a romantic or sexual encounter or relationship with that person.

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