Definitions from Wiktionary (unshackle)
▸ verb: To remove shackles from someone or something.
▸ verb: To remove restrictions or inhibitions; to allow full freedom and power.
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▸ verb: To remove shackles from someone or something.
▸ verb: To remove restrictions or inhibitions; to allow full freedom and power.
Similar:
unbridle,
unmanacle,
unleash,
unfetter,
disencumber,
unharness,
disenthrall,
raise someone's shackles,
uncage,
untie,
more...
Opposite:
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▸ Rhymes of unshackle
▸ Invented words related to unshackle