Usually means: Make smooth or flat again.
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We found 4 dictionaries that define the word uncrumple:

General (4 matching dictionaries)
  1. uncrumple: Merriam-Webster
  2. uncrumple: Oxford Learner's Dictionaries
  3. uncrumple: Collins English Dictionary
  4. uncrumple: Wiktionary

Definitions from Wiktionary (uncrumple)

verb:  (transitive) To return something that has been crumpled closer to its original state.
verb:  (intransitive) Having been crumpled, to return closer to its original state.

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