Usually means: Improves heat transfer between components.
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We found 4 dictionaries that define the word thermal compound:

General (2 matching dictionaries)
  1. thermal compound: Wiktionary
  2. Thermal compound: Wikipedia, the Free Encyclopedia

Computing (2 matching dictionaries)
  1. Webopedia (No longer online)
  2. Thermal compound: Encyclopedia

Definitions from Wiktionary (thermal compound)

noun:  thermal grease

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