Usually means: Prepare lips for a kiss.
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We found 10 dictionaries that define the word pucker up:

General (7 matching dictionaries)
  1. pucker up: Merriam-Webster
  2. pucker up: Oxford Learner's Dictionaries
  3. pucker up: Cambridge Advanced Learner's Dictionary
  4. pucker up: Wiktionary
  5. Pucker Up (disambiguation), Pucker Up, Pucker up: Wikipedia, the Free Encyclopedia

Miscellaneous (1 matching dictionary)
  1. pucker up: Idioms

Slang (2 matching dictionaries)
  1. pucker up: Green’s Dictionary of Slang
  2. pucker up: Urban Dictionary

Definitions from Wiktionary (pucker up)

verb:  (ambitransitive) To contract a facial feature so as to form wrinkles; used especially of the lips when whistling or kissing.

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