Might mean (unverified): Alloy primarily composed of silver, arsenic.
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We found 2 dictionaries that define the word allargentum:

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  1. allargentum: Wiktionary
  2. Allargentum: Wikipedia, the Free Encyclopedia

Definitions from Wiktionary (allargentum)

noun:  (mineralogy) A hexagonal-dihexagonal dipyramidal silver gray mineral containing antimony and silver.

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