Sorry, no online dictionaries contain the exact phrase when two people are in sync.
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Reverse dictionary results:
1. harmony
2. alignment
3. congruence
4. concord
5. rapport
6. accord
7. accordance
8. according
9. commutual
10. compatible
11. concordance
12. concordancy
13. concordant
14. concordial
15. congruous
16. consense
17. consentaneity
18. consistency
19. consistent
20. consonant
21. correspondent
22. en rapport
23. semblable
24. accordant
25. answer
26. concurrence
27. conformable
28. conformably
29. conformity
30. congruency
31. congruent
32. consonancy
33. corresponsive
34. even steven
35. kind
36. match

You can look up the words in the phrase individually using these links:   when ?   two ?   people ?   are ?   in ?   sync ?
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