Sorry, no online dictionaries contain the exact phrase unsettling grin.
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Reverse dictionary results:
1. creepy smile
2. eerie grin
3. unnerving smirk
4. leer
5. sneer
6. creepy
7. eerie
8. nasty
9. stare
10. hair shirt
11. hairy
12. scary
13. ear
14. acne
15. air
16. angry
17. aura
18. bad
19. bat
20. beast
21. bite
22. blare
23. blow
24. bobble
25. boo
26. brace
27. brogue
28. care
29. cat
30. chiller
31. clear
32. cleared
33. courage
34. creep
35. crone
36. cross
37. crown
38. cure
39. cushion
40. darken

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You can look up the words in the phrase individually using these links:   unsettling ?   grin ?
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unse*to search for words beginning with unse, or
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