Sorry, no online dictionaries contain the exact phrase undo a knot.
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Reverse dictionary results:
1. untie
2. untied
3. untying
4. unknot
5. unlaced
6. annul
7. slip
8. tie
9. ravel
10. unlace
11. unlink
12. unlinked
13. unpick
14. unravel
15. unravelling
16. edit
17. eraser
18. ladder
19. loose
20. open
21. ruin
22. solve
23. stand
24. unfasten
25. unweave
26. organize
27. boe
28. burl
29. fasten
30. gordian knot
31. hitch
32. hitching
33. knotting
34. net
35. peanut
36. retie
37. slipknot
38. tippett
39. knothole
40. ablaut

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You can look up the words in the phrase individually using these links:   undo ?   a ?   knot ?
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undo*to search for words beginning with undo, or
*knotto search for words ending with knot
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