Sorry, no online dictionaries contain the exact phrase sure of themselves.
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Reverse dictionary results:
1. confident
2. self-assured
3. assured
4. poised
5. secure
6. perforce
7. sartainty
8. bet
9. fiducially
10. fingers crossed
11. good bet
12. level
13. mandatorily
14. positively
15. seriously
16. soothfastness
17. soothly
18. sure enough
19. almost surely
20. certainly
21. certayne
22. certeine
23. certie
24. cinch
25. confirmedly
26. constat
27. gladly
28. home truth
29. honest to goodness
30. in all probability
31. iwys
32. likely
33. matter of course
34. matter of factly
35. needfulness
36. on the off chance
37. opportunity
38. perchance

You can look up the words in the phrase individually using these links:   sure ?   of ?   themselves ?
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