Sorry, no online dictionaries contain the exact phrase opposite of unwind.
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Reverse dictionary results:
1. wind up
 2. tighten
3. tense
4. coil
5. twist
6. undercut
7. intussuscepted
8. spin out
9. undermine
10. underseal
 11. winddown
12. compress
13. constrict
14. fold up
15. layer
16. overlay
17. riddled
18. turndown
19. circumfuse
20. cutaway
 21. entangle
22. foreshorten
23. indraw
24. intort
25. onlay
26. overshadow
27. revolve
28. rotate
29. run-down
30. steepen
 31. underfoot
32. undergird
33. underlay
34. underset
35. wind down
36. windup
37. cant
38. cap off
39. collapse

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   unwind ?
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