Sorry, no online dictionaries contain the exact phrase opposite of unbutton.
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Reverse dictionary results:
1. button
2. fasten
3. secure
4. close
5. attach
6. do up
7. enfile
8. hasp
9. hook up
10. lace up
11. latch
12. latching
13. lock
14. locke
15. seal
16. stape
17. staple
18. bar
19. barnacle
20. cinch
21. clamp
22. clip
23. cotter
24. deadbolt
25. ferrule
26. grapple
27. hinge
28. jamb
29. lockt
30. padlock
31. pin down
32. rivet
33. spring shackle
34. take up
35. tenon
36. wrap up
37. batten
38. belock

You can look up the words in the phrase individually using these links:   opposite ?   of ?   unbutton ?
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oppo*to search for words beginning with oppo, or
*ttonto search for words ending with tton
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