Sorry, no online dictionaries contain the exact phrase opposite of unbound.
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Reverse dictionary results:
1. bound
2. tied
3. secured
4. fastened
5. secure
6. enfile
7. hook up
8. lace up
9. seal
10. stape
11. staple
12. attach
13. barnacle
14. bind
15. buttress
16. curb
17. curtail
18. do up
19. fasten
20. hasp
21. hinge
22. latch
23. latching
24. lock
25. locke
26. lockt
27. pinnacle
28. stake
29. bar
30. barred
31. buckle
32. buttressed
33. cable
34. chain
35. cinch
36. cotter
37. crutch
38. deadbolt
39. doweled

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   unbound ?
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