Sorry, no online dictionaries contain the exact phrase opposite of simplify.
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Reverse dictionary results:
1. ease
 2. degrade
3. reduce
4. simple
5. streamlined
6. reduced
7. abase
8. again
9. alien
10. bang
 11. bid
12. bonnet
13. bow
14. box
15. boxy
16. cast
17. casted
18. charge
19. charged
20. charging
 21. clash
22. contradict
23. countermine
24. cut
25. difference
26. disinclined
27. down
28. ebb
29. face
30. foul
 31. hit
32. hook
33. however
34. iff
35. imbecile
36. lift
37. loaded
38. luft
39. mar
40. neutralize

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