Sorry, no online dictionaries contain the exact phrase opposite of regularize.
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Reverse dictionary results:
1. irregularize
2. disorganize
3. disorder
4. unsettle
5. disarrange
6. derange
7. disharmonize
8. disjoint
9. disorientate
10. deform
11. destabilise
12. disorganise
13. intemperate
14. uneven
15. destabilize
16. disequilibrate
17. distune
18. untune
19. defuse
20. disarray
21. discompose
22. dishevel
23. distort
24. derangement
25. dislocate
26. disorient
27. dissonate
28. distemper
29. jam
30. unbalance
31. derailment
32. derating
33. disinterest
34. disorganization
35. incapacitated
36. defigure
37. disable

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