Sorry, no online dictionaries contain the exact phrase opposite of loosen up.
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Reverse dictionary results:
1. ease
 2. turnover
3. untie
4. dig
5. relax
6. delve
7. ret
8. delving
9. release
10. oil
 11. reverse
12. scarify
13. unbend
14. chill
15. cut into
16. relaxed
17. slacken
18. thaw
19. turn over
20. untwist
 21. untwisted
22. gad
23. unwind
24. cultivate
25. decompress
26. gsd
27. unlax
28. unstrain
29. unstuff
30. warm
 31. down
32. abed
33. ennui
34. inflation
35. overcompensation
36. free
37. loose
38. shake
39. shaking
40. slack

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   loosen ?   up ?
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Not helpful? You might try using the wildcards * and ? to find the word you're looking for. For example, use
oppo*to search for words beginning with oppo, or
*n upto search for words ending with n up
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