Sorry, no online dictionaries contain the exact phrase opposite of jangled.
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Reverse dictionary results:
1. clash
2. calm
3. discordant
4. placid
5. toned
6. accordant
7. cacophonous
8. confused
9. dissonant
10. peaceful
11. quiet
12. relaxed
13. still
14. jangle
15. jangly
16. attuned
17. cheerful
18. deadened
19. distempered
20. frazzled
21. harp
22. jumbled
23. muddled
24. numbed
25. overstrained
26. overstrung
27. purer
28. serene
29. tortured
30. tranquil
31. untuned
32. ab-
33. abase
34. abe
35. abeam
36. abed
37. abet
38. abhorred
39. aboral
40. about

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   jangled ?
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