Sorry, no online dictionaries contain the exact phrase opposite of align.
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Reverse dictionary results:
1. pull
 2. register
3. side
4. square
5. true
6. aligned
7. ally
8. take
9. guideline
10. jog
 11. line
12. orientate
13. range
14. ranged
15. ranging
16. trie
17. dress
18. tram
19. aim
20. brace
 21. comb
22. commit
23. dowel
24. hike
25. meeting
26. orient
27. oriented
28. orienteering
29. orienting
30. paramagnetism
 31. plumb
32. pulling
33. root
34. abeam
35. abreast
36. again
37. against
38. alternate
39. analysis
40. anti

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You can look up the words in the phrase individually using these links:   opposite ?   of ?   align ?
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oppo*to search for words beginning with oppo, or
*lignto search for words ending with lign
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