Sorry, no online dictionaries contain the exact phrase most vital part.
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Reverse dictionary results:
1. heart
2. core
3. substance
4. essence
5. pith
6. hearts
7. kernel
8. marrow
9. gist
10. meat
11. center
12. sum
13. inwardness
14. nub
15. coring
16. jugular
17. quick
18. centre
19. summing
20. heart and soul
21. nitty-gritty
22. main
23. much
24. soul
25. essentials
26. critical
27. essential
28. key
29. life
30. crucial
31. major
32. principal
33. greater
34. basic
35. fundamental
36. depth
37. mostly
38. central
39. indispensable
40. front

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You can look up the words in the phrase individually using these links:   most ?   vital ?   part ?
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