Sorry, no online dictionaries contain the exact phrase most significantly.
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Reverse dictionary results:
1. primarily
 2. chiefly
3. mainly
4. importantly
5. notably
6. basically
7. by and large
8. largely
9. main
10. majorly
 11. mostly
12. capitally
13. prevalently
14. as a rule
15. capital
16. core
17. essential
18. for the most part
19. imperative
20. maine
 21. mainspring
22. mission-critical
23. more
24. relevant
25. summum bonum
26. superlative degree
27. widely
28. built-in
29. crucial
30. generally
 31. in general
32. instrumental
33. key
34. main thing
35. matter
36. meaningful
37. namely

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