Sorry, no online dictionaries contain the exact phrase most significant accomplishments.

Reverse dictionary results:
1. ultimate
2. greater
3. greatest
4. major
5. more
6. milestones
7. basic
8. highest
9. main
10. paramount
11. top
12. canonical
13. canonic
14. mother
15. anthropocentric
16. bigger
17. biggest
18. crucial
19. essential
20. face
21. foremost
22. gravest
23. heaviest
24. higher
25. important
26. key
27. larger
28. largest
29. lead
30. leading
31. meaningful
32. primary
33. principal
34. principale
35. prominent
36. senior
37. sharper
38. stronger
39. strongest
40. taller

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You can look up the words in the phrase individually using these links:   most ?   significant ?   accomplishments ?
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