Sorry, no online dictionaries contain the exact phrase most mentally sound.
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Reverse dictionary results:
1. sane
2. rational
3. sound-minded
4. clear-headed
5. level-headed
6. fulfilment
7. lucid
8. pliantly
9. auspiciousness
10. civilly
11. cogently
12. conscionably
13. continently
14. disposedly
15. disposedness
16. drivenness
17. gainfulness
18. importance
19. interestingness
20. liberally
21. mattering
22. pendency
23. positiveness
24. procacity
25. publicness
26. responsively
27. sensibly
28. studiousness
29. suasiveness
30. sympathetic
31. temperately
32. tenably
33. towardliness
34. advisably
35. afterness
36. amatively
37. amenities
38. astuteness

You can look up the words in the phrase individually using these links:   most ?   mentally ?   sound ?
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