Sorry, no online dictionaries contain the exact phrase impossibly perfect.
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Reverse dictionary results:
1. ideal
 2. flawless
3. utopian
4. immaculate
5. pristine
6. fair-minded
7. alone
8. casual
9. freeness
10. simple
 11. cleanness
12. guilelessness
13. intransigeance
14. public domain
15. pure
16. simplicity
17. singledom
18. singly
19. solo
20. spotlessness
 21. straightforward
22. candid
23. candor
24. immaculateness
25. impartially
26. inconclusiveness
27. liberality
28. one
29. plain
30. pristinely
 31. pure and simple
32. rarity
33. rigid
34. unpretending
35. voluntarily
36. discretionarily
37. immixed
38. innocency

You can look up the words in the phrase individually using these links:   impossibly ?   perfect ?
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