Sorry, no online dictionaries contain the exact phrase his frown deepened.
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Reverse dictionary results:
1. scowled
2. grimaced
3. glowered
4. scowled deeper
5. frowned more
6. scowl
7. beetle-browed
8. frown
9. gaping
10. gawm
11. gawp
12. glout
13. glower
14. glowering
15. glowr
16. gorm
17. gove
18. grimacing
19. look
20. staring
21. wheezily
22. wincing
23. belgard
24. brinded
25. clum
26. frowning
27. galp
28. gape
29. gaper
30. gapingly
31. gaum
32. gaup
33. gaw
34. gawk
35. gawping
36. gazement
37. glare
38. gloat
39. gloater

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You can look up the words in the phrase individually using these links:   his ?   frown ?   deepened ?
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