Sorry, no online dictionaries contain the exact phrase grand and ambitious.
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Reverse dictionary results:
1. epic
2. expansive
3. grans
4. heroic
5. pretentious
6. saga
7. slam
8. aspire
9. challenging
10. driven
11. flourish
12. harder
13. high-reaching
14. complete
15. era
16. gallant
17. grand tour
18. grat
19. great
20. high
21. sweep
22. think
23. thunk
24. vig
25. vista
26. aim
27. aiming
28. draw a bead on
29. high-pitched
30. hungry
31. praetorian
32. shoot for
33. vanity
34. aaron
35. aeon
36. alcibiades
37. altitudinarian
38. arduous
39. arrant
40. augean

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You can look up the words in the phrase individually using these links:   grand ?   and ?   ambitious ?
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