Sorry, no online dictionaries contain the exact phrase deeply unsettling.
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Reverse dictionary results:
1. disturbing
2. unnerving
3. alarming
4. disconcerting
5. agonizingly
6. botherment
7. bothersome
8. confronting
9. distressful
10. frustrating
11. maddening
12. provoking
13. troublesome
14. troubling
15. achingly
16. aggrievance
17. aggrievedly
18. annoyance
19. annoyedly
20. annoying
21. annoyment
22. anxious
23. bother
24. botheration
25. chagrining
26. crushing
27. disease
28. disheartening
29. dismay
30. dispiritedly
31. disquieting
32. distressing
33. exasperating
34. exasperatingly
35. exasperation
36. excruciatingly
37. frustration
38. frustrative

You can look up the words in the phrase individually using these links:   deeply ?   unsettling ?
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