Sorry, no online dictionaries contain the exact phrase dastardly grin.
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Reverse dictionary results:
1. sneer
2. smirk
3. scowl
4. leer
5. pout
6. pouting
7. powt
8. rictus
9. gawm
10. gren
11. grimacing
12. grin
13. grinning
14. grinny
15. half smile
16. look
17. moue
18. mow
19. mump
20. scowling
21. simper
22. smile
23. smiley
24. smiley face
25. smilie
26. smiling
27. beetle-browed
28. cheesy
29. croakily
30. cynical
31. gaper
32. gaum
33. gawker
34. gern
35. giggly
36. gloater
37. glowering
38. grimace

You can look up the words in the phrase individually using these links:   dastardly ?   grin ?
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dast*to search for words beginning with dast, or
*grinto search for words ending with grin
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