Sorry, no online dictionaries contain the exact phrase achieve harmony of purpose.
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Reverse dictionary results:
1. align
 2. unify
3. harmonize
4. coordinate
5. converge
6. aggregate
7. amalgamate
8. coalesce
9. cofound
10. collate
 11. colligate
12. collude
13. combinate
14. combine
15. compact
16. compaginate
17. compile
18. compound
19. concentrate
20. concentre
 21. concur
22. conglomerate
23. conjoin
24. constellate
25. consubstantiate
26. inosculate
27. accrete
28. add
29. aggregation
30. amass
 31. amassed
32. assort
33. batch
34. bring together
35. coalite
36. cohere

You can look up the words in the phrase individually using these links:   achieve ?   harmony ?   of ?   purpose ?
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