Sorry, no online dictionaries contain the exact phrase act smart.
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Reverse dictionary results:
1. intellect
2. outsmart
3. show off
4. demonstrate intelligence
5. flaunt knowledge
6. busybody
7. lure
8. vaunt
9. wile
10. allure
11. amuse
12. attract
13. attracted
14. attractor
15. avaunt
16. fascinate
17. seduce
18. tantalize
19. toady
20. tole
21. vaunter
22. wheedle
23. bait
24. baiting
25. bribe
26. busy
27. busybodying
28. cajole
29. cajoler
30. cajoling
31. coaxing
32. entice
33. get wise
34. in your face
35. ingratiate
36. inveigle
37. put on airs
38. tempt
39. tempter

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You can look up the words in the phrase individually using these links:   act ?   smart ?
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